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Self-healing, biocompatible, poly(lactide-co-glycolide)-based hydrogel for sustained delivery of acidic payload.
Biocompatible poly(lactide-co-glycolide)-based hydrogels were employed to provide sustained acidic payload delivery in an environment of increased temperature, as seen in human infected wounds. Specifically, polylactic acid (PLA) and poly(D,L-lactide) (PDLLA) were used to form hydrogels for sustained delivery of acidic payloads at pH values of 5.0, 6.0 and 7.0. The structural and degradation properties of these polymers, together with the effect of storage on the gel compositions, were evaluated. The hydrolytic stability of these materials was investigated by preparing samples that were stored in aqueous solution at different temperatures. Results showed that pH 5.0, 6.0 and 7.0 gels degraded at a similar rate over 30 days of storage. Thermal analysis showed that the polymer degradation profiles were similar for PLA and PDLLA at pH values of 5.0, 6.0 and 7.0. Microscopy revealed that the bulk degradation of these materials occurred by surface erosion.
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